Download e-book for kindle: Inorganic Syntheses: v. 11 by William Lee Jolly

By William Lee Jolly

ISBN-10: 0070327637

ISBN-13: 9780070327634

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Additional info for Inorganic Syntheses: v. 11

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Only. of fig. of SOC. of the 3T1 , 3T2 multiplets then shQuld be prQne tQ heavy scrambling by three addi tiQnal, nQn-cQmmuting interactiQns: the crystal field and Jahn-Teller effects, and SOC. olecules. for V043 in YV04 and Ba3(V04) 2 crystals [19J. of the luminescent state. of the iQn expected CONFORMATIONAL CHANGES ON EXCITATION OF TETROXO ANIONS IN CRYSTALS 43 from crystallographic data. The EPR results show that in each of the three systems a lowering of symmetry occurs on excitation. Apparently, the orbi tal degeneracy is lifted and we think the Jahn-Teller instability to be the major cause.

P~(~) ~a ~ --'T]- (8) R. B. GERBER ET AL. 30 1 f dm(~)= ~ 2 2 -1 d1] (9) 2 "b (~ -1] )p,,(1]) ~b d ( )= m 1] f (1_1]2)d~ ~ (~-1])p ~(~) a 2 2 ~b 1 c,,=2f~;c~=f~ (10) ~a p~(~) '1b p,,(1]) It can be shown that the eigenvalues E'mn of the Hamiltonian H' of (3) are within the SCF approximation given by the SCF energies: E'mn = E'm(n) = E'n(m). (11) The energies obtained by solving the SCF equations (5) depend on the parameter a, the focal half-distance parameter of the prolate spheroidal coordinate system (or rather half the distance between the two "centers" from which the H motion is measured.

P~(~) ~a ~ --'T]- (8) R. B. GERBER ET AL. 30 1 f dm(~)= ~ 2 2 -1 d1] (9) 2 "b (~ -1] )p,,(1]) ~b d ( )= m 1] f (1_1]2)d~ ~ (~-1])p ~(~) a 2 2 ~b 1 c,,=2f~;c~=f~ (10) ~a p~(~) '1b p,,(1]) It can be shown that the eigenvalues E'mn of the Hamiltonian H' of (3) are within the SCF approximation given by the SCF energies: E'mn = E'm(n) = E'n(m). (11) The energies obtained by solving the SCF equations (5) depend on the parameter a, the focal half-distance parameter of the prolate spheroidal coordinate system (or rather half the distance between the two "centers" from which the H motion is measured.

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Inorganic Syntheses: v. 11 by William Lee Jolly


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