Read e-book online Molecular Nano Dynamics, Volumes 1-2 PDF

By Hiroshi Fukumura, Masahiro Irie, Yasuhiro Iwasawa, Hiroshi Masuhara, Kohei Uosaki

ISBN-10: 3527320172

ISBN-13: 9783527320172

From man made surfaces to residing cells, Molecular Nano Dynamics, Vol. I and Vol. II explores greater than forty vital tools for dynamic remark of the nanoscale. Edited via absolute technological know-how greats from Japan, this two-volume set covers all vital features of this subject: nanoscale spectroscopy and characterization instruments, nanostructure dynamics, unmarried residing phone dynamics, energetic surfaces, and unmarried crystals. Destined to be the definitive reference paintings on nanoscale molecular dynamics and their commentary for years yet to come, this can be a must-have reference for chemists, physicists, actual chemists, theoretical chemists, and fabrics scientists.

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Furthermore, the light field is enhanced by a factor of $100 or more, depending on the structure and size of the tip apex, due to the resonant effect of the plasmon polaritons. Assuming that the incident field is perpendicular to the incident plane, that is s-polarization, confinement and enhancement of the light field do not occur because the light field oscillating in this direction does not couple with the collective oscillation of electrons at the nano-tip. Even if the incident light field possesses p-polarization, a dielectric or sharpened glass fiber nano-tip exhibits much less confinement and enhancement than a metallic nano-tip.

Nishitani et al. observed the tip-enhanced fluorescence of 8 nm thick meso-tetrakis (3,5-di-tertiarybutyl-phenyl)porphyrin (H2TBPP) films on ITO with an Ag tip [38]. They reported that the fluorescence was enhanced by the locally confined electromagnetic field in the vicinity of the tip. The enhancement factor is evaluated to be larger than 2000. 5 Future Prospects We have reviewed the present situation of research on STM tip-enhanced Raman and fluorescence spectroscopy. There have been several papers showing the enhancement of Raman spectra when tips are in the approached condition.

Briefly, Raman enhancement is considered to occur by two mechanisms: chemical enhancement and electromagnetic enhancement. The chemical enhancement is due to resonance Raman scattering based on charge transfer between a metal nanostructure and a molecule, and takes place only when the metal nanostructure is in contact with the molecule. In STM, the tip is close to the sample molecule but not close enough to induce charge transfer, so the enhancement by the chemical effect may be negligibly small.

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Molecular Nano Dynamics, Volumes 1-2 by Hiroshi Fukumura, Masahiro Irie, Yasuhiro Iwasawa, Hiroshi Masuhara, Kohei Uosaki


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